Funct. Mater. 2022; 29 (4): 481-487.
doi:https://doi.org/10.15407/fm29.04.481
Comparison of luminescent properties of halide perovskite nanocrystals in solutions and polymer films
Institute for Scintillation Materials, National Academy of Sciences of Ukraine, 60 Nauky Ave., 61072 Kharkiv, Ukraine
Abstract:
Halide perovskite nanocrystals of different anion compositions were synthesized using the ligand-assisted reprecipitation method. It has been shown, that toluene is a more suitable solvent compared to chloroform from the point of view of better nanocrystal stability. Chloride perovskites reveal shorter lifetimes but weaker luminescence compared to bromide ones. Embedding perovskite nanocrystals into poly(methyl methacrylate) films leads to a significant shortening the lifetimes of the nanocrystals and much longer stability of the samples. That makes them promising for the creation of fast scintillation materials.
Keywords:
perovskite, nanocrystals, polymer films, luminescence, lifetime, exiton.
References:
| 1. Q.A.Akkerman, G. Raino, M.V.Kovalenko et al., Nat. Mater., 17, 394 (2018). https://doi.org/10.1038/s41563-018-0018-4 |
||||
| 2. A.Dey, J.Ye, A.De et al., ACS Nano, 15, 10775 (2021). https://doi.org/10.1021/acsnano.0c08903 |
||||
| 3. M.V.Kovalenko, L.Protesescu, M.I.Bodnarchuk, Science, 358, 745 (2017). https://doi.org/10.1126/science.aam7093 |
||||
| 4. J.Shamsi, A.S.Urban, M.Imran et al., Chem. Rev., 119, 3296 (2019). https://doi.org/10.1021/acs.chemrev.8b00644 |
||||
| 5. Perovskite Quantum Dots, ed. by Y.Zhou, Y.Wang, Springer Singapore, Singapore (2020). | ||||
| 6. A.L.Efros, L.E.Brus, ACS Nano, 15, 6192 (2021). https://doi.org/10.1021/acsnano.1c01399 |
||||
| 7. N.Wang, W.Liu, Q.Zhang, Small Methods, 2, 1700380 (2018). https://doi.org/10.1002/smtd.201700380 |
||||
| 8. Z.Song, J.Zhao, Q.Liu, Inorg. Chem. Front., 6, 2969 (2019). https://doi.org/10.1039/C9QI00777F |
||||
| 9. Q.Chen, J.Wu, X.Ou et al., Nature, 561, 88 (2018). https://doi.org/10.1038/s41586-018-0451-1 |
||||
| 10. Q.Xu, J.Wang, W.Shao et al., Nanoscale, 12, 9727 (2020). https://doi.org/10.1039/D0NR00772B |
||||
| 11. S.Chhangani, M.Kumar, R.M.Sahani et al., Mater. Today Proc., 48, 1028 (2022). https://doi.org/10.1016/j.matpr.2021.06.432 |
||||
| 12. L.Lu, M.Sun, T.Wu et al., Nanoscale Adv., 4, 680 (2022). https://doi.org/10.1039/D1NA00815C |
||||
| 13. L.Clinckemalie, D.Valli, M.B.J.Roeffaers et al., ACS Energy Lett., 6, 1290 (2021). https://doi.org/10.1021/acsenergylett.1c00007 |
||||
| 14. Z.Zhang, H.Dierks, N.Lamers et al., ACS Appl. Nano Mater., 5, 881 (2022). https://doi.org/10.1021/acsanm.1c03575 |
||||
| 15. C.Dujardin, E.Auffray, E.Bourret-Courchesne et al., IEEE Trans. Nucl. Sci., 65, 1977 (2018). https://doi.org/10.1109/TNS.2018.2840160 |
||||
| 16. P.Lecoq, C.Morel, J.O.Prior et al., Phys. Med. Biol., 65, 21RM01 (2020). https://doi.org/10.1088/1361-6560/ab9500 |
||||
| 17. X.Du, G.Wu, J.Cheng et al., RSC Adv., 7, 10391 (2017). https://doi.org/10.1039/C6RA27665B |
||||
| 18. M.A.Becker, C.Bernasconi, M.I Bodnarchuk et al., ACS Nano, 14, 14939 (2020). https://doi.org/10.1021/acsnano.0c04401 |
||||
| 19. V.S.Chirvony, S.Gonzalez-Carrero, I.Suarez et al., J. Phys. Chem. C, 121, 13381 (2017). https://doi.org/10.1021/acs.jpcc.7b03771 |
||||
| 20. Y.Wang, M.Zhi, Y.Chan, J. Phys. Chem. C, 121, 28498 (2017). https://doi.org/10.1021/acs.jpcc.7b09040 |
||||
| 21. S.J.W.Vonk, M.B.Fridriksson, S.O.M.Hinterding et al., J. Phys. Chem. C, 124, 8047 (2020). https://doi.org/10.1021/acs.jpcc.0c02287 |
||||
| 22. S.K.Gupta, Y.Mao, Front. Optoelectron., 13, 156 (2020). https://doi.org/10.1007/s12200-020-1003-5 |
||||
| 23. R.M.Turtos, S.Gundacker, S.Omelkov et al., Npj 2D Mater. Appl., 3, 37 (2019). https://doi.org/10.1038/s41699-019-0120-8 |
||||
| 24. P.Chen, Z.Xiong, X.Wu et al., J. Phys. Chem. Lett., 8, 3961 (2017). https://doi.org/10.1021/acs.jpclett.7b01562 |
||||
| 25. D.Afanasyev, N.Ibrayev, N.Nuraje, Front. Mater., 7, 600424 (2021). https://doi.org/10.3389/fmats.2020.600424 |
||||
| 26. K.Gu, H.Peng, S.Hua et al., Nanomaterials, 9, 770 (2019). https://doi.org/10.3390/nano9050770 |
||||
| 27. Y.Wu, Q.Han, M.Wang et al., Opt. Express, 29, 36988 (2021). https://doi.org/10.1364/OE.443112 |
||||
| 28. C.-M.Yang, F.-C.Chen, Nanomaterials, 11, 993 (2021). https://doi.org/10.3390/nano11040993 |
||||
| 29. S.Zhang, Y.Liang, Q.Jing et al., Sci. Rep., 7, 14695 (2017). https://doi.org/10.1038/s41598-017-15230-x |
||||
| 30. W.Zhao, Z.Wen, Q.Xu et al., Nanophotonics, 10, 2257 (2021). https://doi.org/10.1515/nanoph-2021-0064 |
||||